Marina Friedel

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Friedel

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Marina

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0000-0001-7739-4691

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Publications 1 - 10 of 14

Exploring the link between austral stratospheric polar vortex anomalies and surface climate in chemistry-climate models
Bergner, Nora; Friedel, Marina; Domeisen, Daniela; et al. (2022)
Atmospheric Chemistry and Physics
Extreme events in the stratospheric polar vortex can lead to changes in the tropospheric circulation and impact the surface climate on a wide range of timescales. The austral stratospheric vortex shows its largest variability in spring, and a weakened polar vortex is associated with changes in the spring to summer surface climate, including hot and dry extremes in Australia. However, the robustness and extent of the connection between polar vortex strength and surface climate on interannual timescales remain unclear. We assess this relationship by using reanalysis data and time-slice simulations from two chemistry-climate models (CCMs), building on previous work that is mainly based on observations. The CCMs show a similar downward propagation of anomalies in the polar vortex strength to the reanalysis data: a weak polar vortex is on average followed by a negative tropospheric Southern Annular Mode (SAM) in spring to summer, while a strong polar vortex is on average followed by a positive SAM. The signature in the surface climate following polar vortex weakenings is characterized by high surface pressure and warm temperature anomalies over Antarctica, the region where surface signals are most robust across all model and observational datasets. However, the tropospheric SAM response in the two CCMs considered is inconsistent with observations. In one CCM, the SAM is more negative compared to the reanalysis after weak polar vortex events, whereas in the other CCM, it is less negative. In addition, neither model reproduces all the regional changes in midlatitudes, such as the warm and dry anomalies over Australia. We find that these inconsistencies are linked to model biases in the basic state, such as the latitude of the eddy-driven jet and the persistence of the SAM. These results are largely corroborated by models that participated in the Chemistry-Climate Model Initiative (CCMI). Furthermore, bootstrapping of the data reveals sizable uncertainty in the magnitude of the surface signals in both models and observations due to internal variability. Our results demonstrate that anomalies of the austral stratospheric vortex have significant impacts on surface climate, although the ability of models to capture regional effects across the Southern Hemisphere is limited by biases in their representation of the stratospheric and tropospheric circulation.
The influence of future changes in springtime Arctic ozone on stratospheric and surface climate
Chiodo, Gabriel; Friedel, Marina; Seeber, Svenja; et al. (2023)
Atmospheric Chemistry and Physics
Stratospheric ozone is expected to recover by the mid-century due to the success of the Montreal Protocol in regulating the emission of ozone-depleting substances (ODSs). In the Arctic, ozone abundances are projected to surpass historical levels due to the combined effect of decreasing ODSs and elevated greenhouse gases (GHGs). While long-term changes in stratospheric ozone have been shown to be a major driver of future surface climate in the Southern Hemisphere during summertime, the dynamical and climatic impacts of elevated ozone levels in the Arctic have not been investigated. In this study, we use two chemistry climate models (the SOlar Climate Ozone Links - Max Planck Ocean Model (SOCOL-MPIOM) and the Community Earth System Model - Whole Atmosphere Community Climate Model (CESM-WACCM)) to assess the climatic impacts of future changes in Arctic ozone on stratospheric dynamics and surface climate in the Northern Hemisphere (NH) during the 21st century. Under the high-emission scenario (RCP8.5) examined in this work, Arctic ozone returns to pre-industrial levels by the middle of the century. Thereby, the increase in Arctic ozone in this scenario warms the lower Arctic stratosphere; reduces the strength of the polar vortex, advancing its breakdown; and weakens the Brewer-Dobson circulation. The ozone-induced changes in springtime generally oppose the effects of GHGs on the polar vortex. In the troposphere, future changes in Arctic ozone induce a negative phase of the Arctic Oscillation, pushing the jet equatorward over the North Atlantic. These impacts of future ozone changes on NH surface climate are smaller than the effects of GHGs, but they are remarkably robust among the two models employed in this study, canceling out a portion of the GHG effects (up to 20% over the Arctic). In the stratosphere, Arctic ozone changes cancel out a much larger fraction of the GHG-induced signal (up to 50 %- 100 %), resulting in no overall change in the projected springtime stratospheric northern annular mode and a reduction in the GHG-induced delay of vortex breakdown of around 15 d. Taken together, our results indicate that future changes in Arctic ozone actively shape the projected changes in the stratospheric circulation and their coupling to the troposphere, thereby playing an important and previously unrecognized role as a driver of the large-scale atmospheric circulation response to climate change.
A global environmental crisis 42,000 years ago
Cooper, Alan; Rozanov, Eugene; Friedel, Marina; et al. (2021)
Science
Geological archives record multiple reversals of Earth’s magnetic poles, but the global impacts of these events, if any, remain unclear. Uncertain radiocarbon calibration has limited investigation of the potential effects of the last major magnetic inversion, known as the Laschamps Excursion [41 to 42 thousand years ago (ka)]. We use ancient New Zealand kauri trees (Agathis australis) to develop a detailed record of atmospheric radiocarbon levels across the Laschamps Excursion. We precisely characterize the geomagnetic reversal and perform global chemistry-climate modeling and detailed radiocarbon dating of paleoenvironmental records to investigate impacts. We find that geomagnetic field minima ~42 ka, in combination with Grand Solar Minima, caused substantial changes in atmospheric ozone concentration and circulation, driving synchronous global climate shifts that caused major environmental changes, extinction events, and transformations in the archaeological record. © 2021 American Association for the Advancement of Science
Global impacts of an extreme solar particle event under different geomagnetic field strengths
Arsenovic, Pavle; Rozanov, Eugene; Usoskin, Ilya; et al. (2024)
Proceedings of the National Academy of Sciences of the United States of America
Solar particle events (SPEs) are short-lived bursts of high-energy particles from the solar atmosphere and are widely recognized as posing significant economic risks to modern society. Most SPEs are relatively weak and have minor impacts on the Earth's environment, but historic records contain much stronger SPEs which have the potential to alter atmospheric chemistry, impacting climate and biological life. The impacts of such strong SPEs would be far more severe when the Earth's protective geomagnetic field is weak, such as during past geomagnetic excursions or reversals. Here, we model the impacts of an extreme SPE under different geomagnetic field strengths, focusing on changes in atmospheric chemistry and surface radiation using the atmosphere-ocean-chemistry-climate model SOCOL3-MPIOM and the radiation transfer model LibRadtran. Under current geomagnetic conditions, an extreme SPE would increase NOx concentrations in the polar stratosphere and mesosphere, causing reductions in extratropical stratospheric ozone lasting for about a year. In contrast, with no geomagnetic field, there would be a substantial increase in NOx throughout the entire atmosphere, resulting in severe stratospheric ozone depletion for several years. The resulting ground-level ultraviolet (UV) radiation would remain elevated for up to 6 y, leading to increases in UV index up to 20 to 25% and solar-induced DNA damage rates by 40 to 50%. The potential evolutionary impacts of past extreme SPEs remain an important question, while the risks they pose to human health in modern conditions continue to be underestimated.
Response to Comment on "A global environmental crisis 42,000 years ago"
Cooper, Alan; Turney, Chris S.M.; Palmer, Jonathan; et al. (2021)
Science
Our study on the exact timing and the potential climatic, environmental, and evolutionary consequences of the Laschamps Geomagnetic Excursion has generated the hypothesis that geomagnetism represents an unrecognized driver in environmental and evolutionary change. It is important for this hypothesis to be tested with new data, and encouragingly, none of the studies presented by Picin et al. undermine our model.
Effects of Arctic ozone on the stratospheric spring onset and its surface impact
Friedel, Marina; Chiodo, Gabriel; Stenke, Andrea; et al. (2022)
Atmospheric Chemistry and Physics
Ozone in the Arctic stratosphere is subject to large interannual variability, driven by both chemical ozone depletion and dynamical variability. Anomalies in Arctic stratospheric ozone become particularly important in spring, when returning sunlight allows them to alter stratospheric temperatures via shortwave heating, thus modifying atmospheric dynamics. At the same time, the stratospheric circulation undergoes a transition in spring with the final stratospheric warming (FSW), which marks the end of winter. A causal link between stratospheric ozone anomalies and FSWs is plausible and might increase the predictability of stratospheric and tropospheric responses on sub-seasonal to seasonal timescales. However, it remains to be fully understood how ozone influences the timing and evolution of the springtime vortex breakdown. Here, we contrast results from chemistry climate models with and without interactive ozone chemistry to quantify the impact of ozone anomalies on the timing of the FSW and its effects on surface climate. We find that ozone feedbacks increase the variability in the timing of the FSW, especially in the lower stratosphere. In ozone-deficient springs, a persistent strong polar vortex and a delayed FSW in the lower stratosphere are partly due to the lack of heating by ozone in that region. High-ozone anomalies, on the other hand, result in additional shortwave heating in the lower stratosphere, where the FSW therefore occurs earlier. We further show that FSWs in high-ozone springs are predominantly followed by a negative phase of the Arctic Oscillation (AO) with positive sea level pressure anomalies over the Arctic and cold anomalies over Eurasia and Europe. These conditions are to a significant extent (at least 50 %) driven by ozone. In contrast, FSWs in low-ozone springs are not associated with a discernible surface climate response. These results highlight the importance of ozone-circulation coupling in the climate system and the potential value of interactive ozone chemistry for sub-seasonal to seasonal predictability.
Atmosphere–ocean–aerosol–chemistry–climate model SOCOLv4.0: description and evaluation
Sukhodolov, Timofei; Egorova, Tatiana; Stenke, Andrea; et al. (2021)
Geoscientific Model Development
This paper features the new atmosphere-ocean-aerosol-chemistry-climate model, SOlar Climate Ozone Links (SOCOL) v4.0, and its validation. The new model was built by interactively coupling the Max Planck Institute Earth System Model version 1.2 (MPI-ESM1.2) (T63, L47) with the chemistry (99 species) and size-resolving (40 bins) sulfate aerosol microphysics modules from the aerosol-chemistry-climate model, SOCOL-AERv2. We evaluate its performance against reanalysis products and observations of atmospheric circulation, temperature, and trace gas distribution, with a focus on stratospheric processes. We show that SOCOLv4.0 captures the low- and midlatitude stratospheric ozone well in terms of the climatological state, variability and evolution. The model provides an accurate representation of climate change, showing a global surface warming trend consistent with observations as well as realistic cooling in the stratosphere caused by greenhouse gas emissions, although, as in previous model versions, a too-fast residual circulation and exaggerated mixing in the surf zone are still present. The stratospheric sulfur budget for moderate volcanic activity is well represented by the model, albeit with slightly underestimated aerosol lifetime after major eruptions. The presence of the interactive ocean and a successful representation of recent climate and ozone layer trends make SOCOLv4.0 ideal for studies devoted to future ozone evolution and effects of greenhouse gases and ozone-destroying substances, as well as the evaluation of potential solar geoengineering measures through sulfur injections. Potential further model improvements could be to increase the vertical resolution, which is expected to allow better meridional transport in the stratosphere, as well as to update the photolysis calculation module and budget of mesospheric odd nitrogen. In summary, this paper demonstrates that SOCOLv4.0 is well suited for applications related to the stratospheric ozone and sulfate aerosol evolution, including its participation in ongoing and future model intercomparison projects.
Stratospherically induced circulation changes under the extreme conditions of the no-Montreal-Protocol scenario
Zilker, Franziska; Sukhodolov, Timofei; Chiodo, Gabriel; et al. (2023)
Atmospheric Chemistry and Physics
The Montreal Protocol and its amendments (MPA) have been a huge success in preserving the stratospheric ozone layer from being destroyed by unabated chlorofluorocarbon (CFC) emissions. The phaseout of CFCs has not only prevented serious impacts on our health and climate, but also avoided strong alterations of atmospheric circulation patterns. With the Earth system model SOCOLv4, we study the dynamical and climatic impacts of a scenario with unabated CFC emissions by 2100, disentangling radiative and chemical (ozone-mediated) effects of CFCs. In the stratosphere, chemical effects of CFCs (i.e., the resulting ozone loss) are the main drivers of circulation changes, weakening wintertime polar vortices and speeding up the Brewer–Dobson circulation. These dynamical impacts during wintertime are due to low-latitude ozone depletion and the resulting reduction in the Equator-to-pole temperature gradient. Westerly winds in the lower stratosphere strengthen, which is for the Southern Hemisphere (SH) similar to the effects of the Antarctic ozone hole over the second half of the 20th century. Furthermore, the winter and spring stratospheric wind variability increases in the SH, whereas it decreases in summer and fall. This seasonal variation in wind speed in the stratosphere has substantial implications for the major modes of variability in the tropospheric circulation in the scenario without the MPA (No-MPA). We find coherent changes in the troposphere, such as patterns that are reminiscent of negative Southern and Northern Annular modes (SAM and NAM) and North Atlantic Oscillation (NAO) anomalies during seasons with a weakened vortex (winter and spring); the opposite occurs during seasons with strengthened westerlies in the lower stratosphere and troposphere (summer). In the troposphere, radiative heating by CFCs prevails throughout the year, shifting the SAM into a positive phase and canceling out the ozone-induced effects on the NAO, whereas the North Pacific sector shows an increase in the meridional sea-level pressure gradient as both CFC heating and ozone-induced effects reinforce each other there. Furthermore, global warming is amplified by 1.7 K with regionally up to a 12 K increase over eastern Canada and the western Arctic. Our study sheds light on the adverse effects of a non-adherence to the MPA on the global atmospheric circulation, uncovering the roles of the underlying physical mechanisms. In so doing, our study emphasizes the importance of the MPA for Earth's climate to avoid regional amplifications of negative climate impacts.
Weakening of springtime Arctic ozone depletion with climate change
Friedel, Marina; Chiodo, Gabriel; Sukhodolov, Timofei; et al. (2023)
Atmospheric Chemistry and Physics
In the Arctic stratosphere, the combination of chemical ozone depletion by halogenated ozone-depleting substances (hODSs) and dynamic fluctuations can lead to severe ozone minima. These Arctic ozone minima are of great societal concern due to their health and climate impacts. Owing to the success of the Montreal Protocol, hODSs in the stratosphere are gradually declining, resulting in a recovery of the ozone layer. On the other hand, continued greenhouse gas (GHG) emissions cool the stratosphere, possibly enhancing the formation of polar stratospheric clouds (PSCs) and, thus, enabling more efficient chemical ozone destruction. Other processes, such as the acceleration of the Brewer–Dobson circulation, also affect stratospheric temperatures, further complicating the picture. Therefore, it is currently unclear whether major Arctic ozone minima will still occur at the end of the 21st century despite decreasing hODSs. We have examined this question for different emission pathways using simulations conducted within the Chemistry-Climate Model Initiative (CCMI-1 and CCMI-2022) and found large differences in the models' ability to simulate the magnitude of ozone minima in the present-day climate. Models with a generally too-cold polar stratosphere (cold bias) produce pronounced ozone minima under present-day climate conditions because they simulate more PSCs and, thus, high concentrations of active chlorine species (ClOₓ). These models predict the largest decrease in ozone minima in the future. Conversely, models with a warm polar stratosphere (warm bias) have the smallest sensitivity of ozone minima to future changes in hODS and GHG concentrations. As a result, the scatter among models in terms of the magnitude of Arctic spring ozone minima will decrease in the future. Overall, these results suggest that Arctic ozone minima will become weaker over the next decades, largely due to the decline in hODS abundances. We note that none of the models analysed here project a notable increase of ozone minima in the future. Stratospheric cooling caused by increasing GHG concentrations is expected to play a secondary role as its effect in the Arctic stratosphere is weakened by opposing radiative and dynamical mechanisms.
Weakening of springtime Arctic ozone depletion with climate change
Friedel, Marina; Chiodo, Gabriel; Peter, Thomas (2023)
EGUsphere
Arctic ozone is subject to large interannual variability, and severe ozone minima can occur through chemical ozone depletion and dynamical variability. Such Arctic ozone minima have been shown to bear a great societal relevance due to their impacts on health and climate. Following the success of the Montreal Protocol, ozone depleting substances (ODSs) in the stratosphere are declining, implying an expected weakening of chemical ozone destruction. However, continuing greenhouse gas (GHG) emissions cool the stratosphere, which might lead to an enhanced formation of polar stratospheric clouds (PSCs) and thus more efficient chemical depletion of ozone. Due to these opposing processes, there is currently no consensus on the fate of Arctic ozone minima in future climate. Here, we investigate the future evolution of Arctic ozone minima over the 21st century under different emission pathways in simulations conducted for the Chemistry-Climate Model Initiative (CCMI), CCMI-1 and CCMI-2022, and constrain these projections based on the models’ skill in reproducing present-day Arctic ozone variability. We find a large model discrepancy in the magnitude of ozone minima under present-day climate, caused by biases in the underlying model climatology. Models that simulate large ozone minima in present-day climate generally have a cold bias, and consequently large concentrations of active chlorine species (ClOx); these are the models that project the largest decline in the magnitude of ozone minima in the future. Conversely, models simulating weak Arctic ozone minima under present-day conditions generally have a warm bias and small ClOx concentrations; these are models with the smallest sensitivity of ozone minima to changes in ODS and GHG emissions. Consequently, inter-model spread in the magnitude of springtime Arctic ozone minima is projected to decline in the future. Through comparison with reanalysis, we identify the most realistic models. These models show a weakening in stratospheric ozone minima of about 1 DU/decade and with little sensitivity to the GHG emission scenario, which is deemed as the most likely projection. Taken together, these results indicate that Arctic ozone minima will likely become weaker in the future, largely due to the decline in ODS abundances, while stratospheric cooling due to GHGs is expected to play a secondary role.

Publications 1 - 10 of 14

Marina Friedel

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