Enhanced Chiral Sensing with Dielectric Nanoresonators


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Date

2020-01-08

Publication Type

Journal Article

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Abstract

Chiro-sensitive molecular detection is highly relevant as many biochemical compounds, the building blocks of life, are chiral. Optical chirality is conventionally detected through circular dichroism (CD) in the UV range, where molecules naturally absorb. Recently, plasmonics has been proposed as a way to boost the otherwise very weak CD signal and translate it to the visible/NIR range, where technology is friendlier. Here, we explore how dielectric nanoresonators can contribute to efficiently differentiate molecular enantiomers. We study the influence of the detuning between electric (ED) and magnetic dipole (MD) resonances in silicon nanocylinders on the quality of the CD signal. While our experimental data, supported by numerical simulations, demonstrate that dielectric nanoresonators can perform even better than their plasmonic counterpart, exhibiting larger CD enhancements, we do not observe any significant influence of the optical chirality. © 2019 American Chemical Society.

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published

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Volume

20 (1)

Pages / Article No.

585 - 591

Publisher

American Chemical Society

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Subject

Bionanophotonics; Chirality; Biosensing; Dielectric nanoresonators; Circular dichroism; Nano-optics

Organisational unit

09698 - Quidant, Romain / Quidant, Romain check_circle

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