Cobalt-Catalyzed Aerobic Aminocyclization of Unsaturated Amides for the Synthesis of Functionalized γ- and δ-Lactams


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Date

2023-09-01

Publication Type

Journal Article

ETH Bibliography

yes

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Abstract

We report the cobalt-catalyzed aminocyclization of unsaturated N-acyl sulfonamides in the presence of oxygen to provide γ- and δ-lactam aldehydes. Use of an optically active cobalt catalyst resulted in the formation of enantiomerically enriched γ-and δ-lactam alcohols. The γ-lactam aldehydes and alcohols obtained were elaborated into useful building blocks.

Publication status

published

Editor

Book title

Volume

25 (34)

Pages / Article No.

6380 - 6384

Publisher

American Chemical Society

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Edition / version

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Geographic location

Date collected

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Subject

Organisational unit

03511 - Carreira, Erick M. / Carreira, Erick M. check_circle

Notes

Funding

833540 - Development of Stereoselective Olefin Functionalization Methods (EC)

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