Synergism of anisotropic and computational NMR methods reveals the likely configuration of phormidolide A


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Date

2020-07-14

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Journal Article

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Abstract

Characterization of the complex molecular scaffold of the marine polyketide natural product phormidolide A represents a challenge that has persisted for nearly two decades. In light of discordant results arising from recent synthetic and biosynthetic reports, a rigorous study of the configuration of phormidolide A was necessary. This report outlines a synergistic effort employing computational and anisotropic NMR investigation, that provided orthogonal confirmation of the reassigned side chain, as well as supporting a further correction of the C7 stereocenter. © 2020 The Royal Society of Chemistry

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published

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56 (55)

Pages / Article No.

7565 - 7568

Publisher

Royal Society of Chemistry

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03980 - Piel, Jörn / Piel, Jörn check_circle

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