PdCu supported on dendritic mesoporous CexZr1-xO2 as superior catalysts to boost CO2 hydrogenation to methanol


METADATA ONLY
Loading...

Date

2022-04

Publication Type

Journal Article

ETH Bibliography

no

Citations

Altmetric
METADATA ONLY

Data

Rights / License

Abstract

A dendritic PdCu/Ce0.3Zr0.7O2 (PdCu/CZ-3) catalyst with uniform spherical morphology was prepared for boosting the catalytic performance of CO2 hydrogenation to methanol (MeOH). The open dendritic pore channels and small particle sizes could reduce not only the diffuse resistance of reactants and products but also increase the accessibility between the active sites (PdCu and oxygen vacancy) and the reactants (H2 and CO2). More spillover hydrogen could be generated due to the highly dispersed PdCu active metals over the PdCu/CZ-3 catalyst. PdCu/CZ-3 can stimulate the generation of more Ce3+ cations, which is beneficial to produce more oxygen vacancies on the surface of the CZ-3 composite. Spillover hydrogen and oxygen vacancy could promote the formate and methoxy routes over PdCu/CZ-3, the primary intermediates producing MeOH. PdCu/CZ-3 displayed the highest CO2 conversions (25.5 %), highest MeOH yield (6.4 %), highest PdCu-TOFMeOH (7.7 h−1) and superior 100 h long-term stability than those of other PdCu/CexZr1-xO2 analogs and the reference PdCu/CeO2 and PdCu/ZrO2 catalysts. Density functional theory (DFT) calculations and in situ DRIFTS were performed to investigate the CO2 − MeOH hydrogenation mechanism.

Publication status

published

Editor

Book title

Volume

611

Pages / Article No.

739 - 751

Publisher

Elsevier

Event

Edition / version

Methods

Software

Geographic location

Date collected

Date created

Subject

Organisational unit

02293 - Catalysis Hub / Catalysis Hub

Notes

Funding

Related publications and datasets