Ultrahigh-throughput screening enables efficient single-round oxidase remodelling


Loading...

Date

2019-09

Publication Type

Journal Article

ETH Bibliography

yes

Citations

Altmetric

Data

Abstract

Biocatalysis provides a potentially sustainable means of chemical manufacturing. However, the tailoring of enzymes to industrial processes is often laborious and time consuming, which limits the broad implementation of this approach. High-throughput screening methods can expedite the search for suitable catalysts, but are often constrained by the need for labelled substrates. The generalization of such techniques would therefore significantly expand their impact. Here we have established a versatile ultrahigh-throughput microfluidic assay that enables isolation of functional oxidases from libraries that contain up to 107 members. The increased throughput over prevalent methods led to complete active-site remodelling of cyclohexylamine oxidase in one round of directed evolution. A 960-fold increase in catalytic efficiency afforded an enzyme with wild-type levels of activity for a non-natural substrate, allowing biocatalytic synthesis of a sterically demanding pharmaceutical intermediate with complete stereocontrol. The coupled enzyme assay is label free and can be easily adapted to re-engineer any oxidase.

Publication status

published

Editor

Book title

Volume

2 (9)

Pages / Article No.

740 - 747

Publisher

Nature

Event

Edition / version

Methods

Software

Geographic location

Date collected

Date created

Subject

Asymmetric catalysis; Biocatalysis; High-throughput screening; Oxidoreductase

Organisational unit

03492 - Hilvert, Donald (emeritus) / Hilvert, Donald (emeritus) check_circle

Notes

It was possible to publish this article open access thanks to a Swiss National Licence with the publisher.

Funding

Related publications and datasets