Template Stripping of Perovskite Thin Films for Dry Interfacing and Surface Structuring
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Date
2020-06-10
Publication Type
Journal Article
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Abstract
Combining excellent optoelectronic properties with the benefits of solution processability, metal-halide perovskites are promising materials for photovoltaic and light-emitting technologies. To facilitate the integration of perovskite thin films into optoelectronic devices, a need exists for simple and efficient fabrication methods. Here, we present a template-stripping technique to produce ultraflat and flexible perovskite thin films. We apply a one-step spin-coating procedure to produce high-quality CH3NH3PbBr3 perovskite thin films on top of ultraflat silicon templates. These films can be mechanically cleaved from the template using a polymer adhesive to reveal the ultraflat perovskite surfaces. We demonstrate how the flatness and flexibility of the template-stripped films enable new processing strategies based on dry interfacing, by interfacing them with plasmonic hole arrays. Moreover, we show that by using prepatterned silicon templates, structured perovskite surfaces can be produced with feature sizes down to a micrometer.
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published
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Journal / series
Volume
12 (23)
Pages / Article No.
26601 - 26606
Publisher
American Chemical Society
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Subject
Perovskite; Template stripping; Thin film; Interface; Flexibility
Organisational unit
03875 - Norris, David J. / Norris, David J.
Notes
Funding
339905 - Quantum-Dot Plasmonics and Spasers (EC)