Electron Scattering in Liquid Water and Amorphous Ice: A Striking Resemblance
dc.contributor.author
Signorell, Ruth
dc.date.accessioned
2020-04-29T09:12:08Z
dc.date.available
2020-04-28T16:04:30Z
dc.date.available
2020-04-29T09:12:08Z
dc.date.issued
2020-03-31
dc.identifier.uri
http://hdl.handle.net/20.500.11850/412152
dc.identifier.doi
10.3929/ethz-b-000412152
dc.description.abstract
The lack of accurate low-energy electron scattering cross sections for liquid water is a substantial source of uncertainty in the modelling of radiation chemistry and biology. The use of existing amorphous ice scattering cross sections for lack of liquid data has been discussed controversially over decades. Here, we compare experimental photoemission data of liquid water with corresponding predictions using amorphous ice cross sections, with the aim of resolving the debate regarding the difference of electron scattering in liquid water and amorphous ice. We find very similar scattering properties in the liquid and the ice for electron kinetic energies up to a few hundred electron volts. The scattering cross sections recommended here for liquid water are an extension of the amorphous ice cross sections. Within the framework of currently available experimental data, our work answers one of the most debated questions regarding electron scattering in liquid water.
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dc.format
application/pdf
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dc.language.iso
en
en_US
dc.publisher
ETH Zurich
en_US
dc.rights.uri
http://rightsstatements.org/page/InC-NC/1.0/
dc.title
Electron Scattering in Liquid Water and Amorphous Ice: A Striking Resemblance
en_US
dc.type
Working Paper
dc.rights.license
In Copyright - Non-Commercial Use Permitted
ethz.pages.start
2003.14008
en_US
ethz.size
21 p.
en_US
ethz.notes
Published in Arxiv
en_US
ethz.grant
Droplet Photoelectron Imaging
en_US
ethz.grant
Molecular Ultrafast Science and Technology (MUST)
en_US
ethz.grant
Phase Transitions of Ultrafine Aerosol Particles: Condensation, Freezing, and Metal Formation in Confined Systems
en_US
ethz.publication.place
Zurich
en_US
ethz.publication.status
published
en_US
ethz.leitzahl
ETH Zürich::00002 - ETH Zürich::00012 - Lehre und Forschung::00007 - Departemente::02020 - Dep. Chemie und Angewandte Biowiss. / Dep. of Chemistry and Applied Biosc.::02515 - Laboratorium für Physikalische Chemie / Laboratory of Physical Chemistry::03961 - Signorell, Ruth / Signorell, Ruth
en_US
ethz.leitzahl.certified
ETH Zürich::00002 - ETH Zürich::00012 - Lehre und Forschung::00007 - Departemente::02020 - Dep. Chemie und Angewandte Biowiss. / Dep. of Chemistry and Applied Biosc.::02515 - Laboratorium für Physikalische Chemie / Laboratory of Physical Chemistry::03961 - Signorell, Ruth / Signorell, Ruth
en_US
ethz.grant.agreementno
786636
ethz.grant.agreementno
125760
ethz.grant.agreementno
172472
ethz.grant.fundername
EC
ethz.grant.fundername
SNF
ethz.grant.fundername
SNF
ethz.grant.funderDoi
10.13039/501100000780
ethz.grant.funderDoi
10.13039/501100001711
ethz.grant.funderDoi
10.13039/501100001711
ethz.grant.program
H2020
ethz.grant.program
NCCR full proposal
ethz.grant.program
Projekte MINT
ethz.relation.isPreviousVersionOf
10.3929/ethz-b-000416314
ethz.date.deposited
2020-04-28T16:04:38Z
ethz.source
FORM
ethz.eth
yes
en_US
ethz.availability
Open access
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ethz.rosetta.installDate
2020-04-29T09:12:19Z
ethz.rosetta.lastUpdated
2022-03-29T01:54:38Z
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