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dc.contributor.author
Jetzki, Martin
dc.contributor.author
Bonnamy, Anthony
dc.contributor.author
Signorell, Ruth
dc.date.accessioned
2020-07-31T04:51:25Z
dc.date.available
2020-07-30T14:16:03Z
dc.date.available
2020-07-31T04:51:25Z
dc.date.issued
2004
dc.identifier.issn
0021-9606
dc.identifier.issn
1089-7690
dc.identifier.other
10.1063/1.1752889
en_US
dc.identifier.uri
http://hdl.handle.net/20.500.11850/429315
dc.identifier.doi
10.3929/ethz-b-000429315
dc.description.abstract
The present contribution investigates shape effects and surface effects in the infrared spectra of pure (NH3) and mixed ( NH3–CO2 and NH3–NH2D–NHD2–ND3) ammonia particles with sizes between about 1 and 50 nm. The particles investigated have been generated in a collisional cooling cell as aerosols at temperatures between 20 and 80 K. The contribution reveals that only the combination with a microscopic model leads to a comprehensive understanding of the various features observed in the experimental infrared spectra. As one of the major results, the corresponding exciton model explains why pronounced shape effects observed for pure particles only play a minor role in the case of mixed particles.
en_US
dc.format
application/pdf
en_US
dc.language.iso
en
en_US
dc.publisher
AIP Publishing
en_US
dc.rights.uri
http://rightsstatements.org/page/InC-NC/1.0/
dc.title
Vibrational delocalization in ammonia aerosol particles
en_US
dc.type
Journal Article
dc.rights.license
In Copyright - Non-Commercial Use Permitted
dc.date.published
2004-06-08
ethz.journal.title
The Journal of Chemical Physics
ethz.journal.volume
120
en_US
ethz.journal.issue
24
en_US
ethz.journal.abbreviated
J. Chem. Phys.
ethz.pages.start
11775
en_US
ethz.pages.end
11784
en_US
ethz.size
10 p.
en_US
ethz.version.deposit
publishedVersion
en_US
ethz.publication.place
College Park, MD
en_US
ethz.publication.status
published
en_US
ethz.leitzahl
ETH Zürich::00002 - ETH Zürich::00012 - Lehre und Forschung::00007 - Departemente::02020 - Dep. Chemie und Angewandte Biowiss. / Dep. of Chemistry and Applied Biosc.::02515 - Laboratorium für Physikalische Chemie / Laboratory of Physical Chemistry::03961 - Signorell, Ruth / Signorell, Ruth
en_US
ethz.leitzahl.certified
ETH Zürich::00002 - ETH Zürich::00012 - Lehre und Forschung::00007 - Departemente::02020 - Dep. Chemie und Angewandte Biowiss. / Dep. of Chemistry and Applied Biosc.::02515 - Laboratorium für Physikalische Chemie / Laboratory of Physical Chemistry::03961 - Signorell, Ruth / Signorell, Ruth
en_US
ethz.date.deposited
2020-07-30T14:16:13Z
ethz.source
FORM
ethz.eth
no
en_US
ethz.availability
Open access
en_US
ethz.rosetta.installDate
2020-07-31T04:51:44Z
ethz.rosetta.lastUpdated
2022-03-29T02:43:54Z
ethz.rosetta.versionExported
true
ethz.COinS
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