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dc.contributor.author
Kesselring, Tobias A.
dc.contributor.author
Franzese, Giancarlo
dc.contributor.author
Buldyrev, Sergey V.
dc.contributor.author
Herrmann, Hans J.
dc.contributor.author
Stanley, H. Eugene
dc.date.accessioned
2018-09-10T15:57:00Z
dc.date.available
2017-06-10T02:06:25Z
dc.date.available
2018-09-10T15:57:00Z
dc.date.issued
2012-06
dc.identifier.other
10.1038/srep00474
en_US
dc.identifier.uri
http://hdl.handle.net/20.500.11850/51333
dc.identifier.doi
10.3929/ethz-b-000051333
dc.description.abstract
One hypothesized explanation for water's anomalies imagines the existence of a liquid-liquid (LL) phase transition line separating two liquid phases and terminating at a LL critical point. We simulate the classic ST2 model of water for times up to 1000 ns and system size up to N = 729. We find that for state points near the LL transition line, the entire system flips rapidly between liquid states of high and low density. Our finite-size scaling analysis accurately locates both the LL transition line and its associated LL critical point. We test the stability of the two liquids with respect to the crystal and find that of the 350 systems simulated, only 3 of them crystallize and these 3 for the relatively small system size N = 343 while for all other simulations the incipient crystallites vanish on a time scales smaller than ≈ 100 ns.
en_US
dc.format
application/pdf
en_US
dc.language.iso
en
en_US
dc.publisher
Nature Publishing Group
en_US
dc.rights.uri
http://creativecommons.org/licenses/by-nc-sa/3.0/
dc.subject
Theoretical physics
en_US
dc.subject
Theoretical chemistry
en_US
dc.subject
Statistical physics, thermodynamics and nonlinear dynamics
en_US
dc.subject
Applied physics
en_US
dc.title
Nanoscale Dynamics of Phase Flipping in Water near its Hypothesized Liquid-Liquid Critical Point
en_US
dc.type
Journal Article
dc.rights.license
Creative Commons Attribution-NonCommercial-ShareAlike 3.0 Unported
ethz.journal.title
Scientific Reports
ethz.journal.volume
2
en_US
ethz.pages.start
474
en_US
ethz.size
6 p.
en_US
ethz.version.deposit
publishedVersion
en_US
ethz.identifier.wos
ethz.identifier.scopus
ethz.identifier.nebis
006751867
ethz.publication.place
London
en_US
ethz.publication.status
published
en_US
ethz.leitzahl
ETH Zürich::00002 - ETH Zürich::00012 - Lehre und Forschung::00007 - Departemente::02115 - Dep. Bau, Umwelt und Geomatik / Dep. of Civil, Env. and Geomatic Eng.::02606 - Institut für Baustoffe (IfB) / Institute for Building Materials::03733 - Herrmann, Hans Jürgen (emeritus) / Herrmann, Hans Jürgen (emeritus)
en_US
ethz.leitzahl.certified
ETH Zürich::00002 - ETH Zürich::00012 - Lehre und Forschung::00007 - Departemente::02115 - Dep. Bau, Umwelt und Geomatik / Dep. of Civil, Env. and Geomatic Eng.::02606 - Institut für Baustoffe (IfB) / Institute for Building Materials::03733 - Herrmann, Hans Jürgen (emeritus) / Herrmann, Hans Jürgen (emeritus)
ethz.date.deposited
2017-06-10T02:06:28Z
ethz.source
ECIT
ethz.identifier.importid
imp59364f66b153d80221
ethz.ecitpid
pub:83793
ethz.eth
yes
en_US
ethz.availability
Open access
en_US
ethz.rosetta.installDate
2017-07-12T11:06:23Z
ethz.rosetta.lastUpdated
2019-02-03T07:50:37Z
ethz.rosetta.exportRequired
true
ethz.rosetta.versionExported
true
ethz.COinS
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