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dc.contributor.author
Donat, Felix
dc.contributor.author
Kierzkowska, Agnieszka
dc.contributor.author
Müller, Christoph R.
dc.date.accessioned
2023-07-31T09:12:45Z
dc.date.available
2022-07-28T03:20:55Z
dc.date.available
2022-07-29T10:43:52Z
dc.date.available
2022-09-07T09:35:11Z
dc.date.available
2023-06-15T20:19:42Z
dc.date.available
2023-06-16T06:24:15Z
dc.date.available
2023-06-16T06:32:32Z
dc.date.available
2023-07-14T12:24:19Z
dc.date.available
2023-07-31T09:12:45Z
dc.date.issued
2022-09-01
dc.identifier.issn
0887-0624
dc.identifier.issn
1520-5029
dc.identifier.other
10.1021/acs.energyfuels.2c01345
en_US
dc.identifier.uri
http://hdl.handle.net/20.500.11850/560507
dc.identifier.doi
10.3929/ethz-b-000560507
dc.description.abstract
In chemical looping, Fe-containing oxygen carriers can catalyze as a side reaction the decomposition of methane, which results in the deposition of carbon on their surface with multiple adverse effects. In this work, we propose a strategy to reduce the extent of carbon deposition by using Co as a second redox-active metal that forms a bimetallic phase with Fe during reduction. We show for a perovskite-based oxygen carrier that the formation of the bimetallic Fe-Co phase improves the dispersion and decreases the size of iron within the material, which may influence its catalytic effect on the decomposition of methane (in addition to potential changes in its electronic structure).
en_US
dc.format
application/pdf
en_US
dc.language.iso
en
en_US
dc.publisher
American Chemical Society
en_US
dc.rights.uri
http://rightsstatements.org/page/InC-NC/1.0/
dc.title
Chemical Looping Partial Oxidation of Methane: Reducing Carbon Deposition through Alloying
en_US
dc.type
Journal Article
dc.rights.license
In Copyright - Non-Commercial Use Permitted
dc.date.published
2022-07-07
ethz.journal.title
Energy & Fuels
ethz.journal.volume
36
en_US
ethz.journal.issue
17
en_US
ethz.journal.abbreviated
Energy Fuels
ethz.pages.start
9780
en_US
ethz.pages.end
9784
en_US
ethz.version.deposit
acceptedVersion
en_US
ethz.grant
Advancing CO2 Capture Materials by Atomic Scale Design: the Quest for Understanding
en_US
ethz.grant
NCCR Catalysis (phase I)
en_US
ethz.identifier.wos
ethz.identifier.scopus
ethz.publication.place
Washington, DC
en_US
ethz.publication.status
published
en_US
ethz.leitzahl
ETH Zürich::00002 - ETH Zürich::00012 - Lehre und Forschung::00007 - Departemente::02130 - Dep. Maschinenbau und Verfahrenstechnik / Dep. of Mechanical and Process Eng.::02668 - Inst. f. Energie- und Verfahrenstechnik / Inst. Energy and Process Engineering::03865 - Müller, Christoph R. / Müller, Christoph R.
en_US
ethz.leitzahl.certified
ETH Zürich::00002 - ETH Zürich::00012 - Lehre und Forschung::00007 - Departemente::02130 - Dep. Maschinenbau und Verfahrenstechnik / Dep. of Mechanical and Process Eng.::02668 - Inst. f. Energie- und Verfahrenstechnik / Inst. Energy and Process Engineering::03865 - Müller, Christoph R. / Müller, Christoph R.
ethz.grant.agreementno
819573
ethz.grant.agreementno
180544
ethz.grant.fundername
EC
ethz.grant.fundername
SNF
ethz.grant.funderDoi
10.13039/501100000780
ethz.grant.funderDoi
10.13039/501100001711
ethz.grant.program
H2020
ethz.grant.program
NCCR full proposal
ethz.date.deposited
2022-07-28T03:21:22Z
ethz.source
WOS
ethz.eth
yes
en_US
ethz.availability
Open access
en_US
ethz.date.embargoend
2023-07-07
ethz.rosetta.installDate
2022-09-07T09:35:17Z
ethz.rosetta.lastUpdated
2024-02-03T02:10:10Z
ethz.rosetta.exportRequired
true
ethz.rosetta.versionExported
true
ethz.COinS
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