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dc.contributor.author
Marx, Dorian
dc.contributor.author
Joss, Lisa
dc.contributor.author
Casas, Nathalie
dc.contributor.author
Schell, Johanna
dc.contributor.author
Mazzotti, Marco
dc.date.accessioned
2021-05-07T12:30:31Z
dc.date.available
2017-06-11T00:29:51Z
dc.date.available
2019-11-01T14:39:33Z
dc.date.available
2021-05-07T12:30:31Z
dc.date.issued
2014-02
dc.identifier.issn
0929-5607
dc.identifier.issn
1572-8757
dc.identifier.other
10.1007/s10450-013-9593-5
en_US
dc.identifier.uri
http://hdl.handle.net/20.500.11850/75109
dc.identifier.doi
10.3929/ethz-b-000075109
dc.description.abstract
The results of breakthrough experiments in an adsorption column packed with commercial activated carbon for three binary CO2/N2 mixtures as well as for two ternary CO2/N2/H2 mixtures are presented. The experiments were carried out at two different temperatures (25 and 45 °C), four different pressures (1, 5, 10 and 20 bar) and three different flow rates. To analyze the experiments, the breakthrough profiles are simulated using a one-dimensional model consisting of material and energy balances together with the necessary constitutive equations. Transport parameters such as the heat and mass transfer coefficients are fitted to the results from the experiments with the binary mixtures (CO2/N2) and then compared to parameters obtained in a previous work (Adsorption 18: 143–161, 2012) for binary CO2/H2 mixtures. Furthermore, the parameters obtained for binary mixtures are used to predict the outcome of breakthrough experiments with ternary CO2/N2/H2 mixtures. These simulations are then tested by experiments, showing that their prediction capability is rather satisfactory for a large range of experimental conditions.
en_US
dc.format
application/pdf
en_US
dc.language.iso
en
en_US
dc.publisher
Springer
en_US
dc.rights.uri
http://rightsstatements.org/page/InC-NC/1.0/
dc.subject
Ternary breakthrough experiments
en_US
dc.subject
Transport parameter estimation
en_US
dc.subject
Fixed bed modeling
en_US
dc.subject
Activated carbon
en_US
dc.subject
CO2 capture
en_US
dc.title
Prediction of non-isothermal ternary gas-phase breakthrough experiments based on binary data
en_US
dc.type
Journal Article
dc.rights.license
In Copyright - Non-Commercial Use Permitted
dc.date.published
2013-11-29
ethz.journal.title
Adsorption
ethz.journal.volume
20
en_US
ethz.journal.issue
2-3
en_US
ethz.journal.abbreviated
Adsorption
ethz.pages.start
493
en_US
ethz.pages.end
510
en_US
ethz.version.deposit
publishedVersion
en_US
ethz.notes
It was possible to publish this article open access thanks to a Swiss National Licence with the publisher.
en_US
ethz.identifier.wos
ethz.identifier.scopus
ethz.publication.place
Berlin
en_US
ethz.publication.status
published
en_US
ethz.leitzahl
ETH Zürich::00002 - ETH Zürich::00012 - Lehre und Forschung::00007 - Departemente::02130 - Dep. Maschinenbau und Verfahrenstechnik / Dep. of Mechanical and Process Eng.::02668 - Inst. f. Energie- und Verfahrenstechnik / Inst. Energy and Process Engineering::03484 - Mazzotti, Marco / Mazzotti, Marco
en_US
ethz.leitzahl.certified
ETH Zürich::00002 - ETH Zürich::00012 - Lehre und Forschung::00007 - Departemente::02130 - Dep. Maschinenbau und Verfahrenstechnik / Dep. of Mechanical and Process Eng.::02668 - Inst. f. Energie- und Verfahrenstechnik / Inst. Energy and Process Engineering::03484 - Mazzotti, Marco / Mazzotti, Marco
ethz.date.deposited
2017-06-11T00:30:56Z
ethz.source
ECIT
ethz.identifier.importid
imp5936513c7c6b348841
ethz.ecitpid
pub:118713
ethz.eth
yes
en_US
ethz.availability
Open access
en_US
ethz.rosetta.installDate
2017-07-14T17:42:34Z
ethz.rosetta.lastUpdated
2022-03-29T07:09:43Z
ethz.rosetta.versionExported
true
ethz.COinS
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