Jamie Massey
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- Investigating skyrmion stability and core polarity reversal in NdMn2Ge2Item type: Journal Article
Scientific ReportsTreves, Samuel K.; Ukleev, Victor; Apseros, Andreas; et al. (2025)We present a study on nanoscale skyrmionic spin textures in NdMn2Ge2, a rare-earth complex noncollinear ferromagnet. We confirm, using X-ray microscopy, that NdMn2Ge2 can host lattices of metastable skyrmion bubbles at room temperature in the absence of a magnetic field, after applying a suitable field cooling protocol. The skyrmion bubbles are robust against temperature changes from room temperature to 330 K. Furthermore, the skyrmion bubbles can be distorted, deformed, and recovered by varying strength and orientation of the applied magnetic field. We have used nitrogen vacancy nanoscale magnetic imaging to estimate and map the magnetic stray fields originating from our NdMn2Ge2 lamella samples and find stray field magnitudes on the order of a few mT near the sample surface. Micromagnetic simulations show an overall agreement with the observed behaviour of the sample under different magnetic field protocols. We also find that the presence of the Dzyaloshinskii-Moriya interaction is not required to reproduce our experimental results. Its inclusion in the simulation leads to a reversal of the skyrmionic object core polarity, which is not experimentally observed. Our results further corroborate the stability and robustness of the skyrmion bubbles formed in NdMn2Ge2 and their potential for future spintronic applications. - X-ray imaging of the magnetic configuration of a three-dimensional artificial spin ice building blockItem type: Journal Article
APL MaterialsPip, Petai; Treves, Samuel; Massey, Jamie; et al. (2022)The extension of artificial spin systems to the third dimension offers advances in functionalities and opportunities for technological applications. One of the main challenges facing their realization is the fabrication of three-dimensional geometries with nanoscale resolution. In this work, we combine two-photon lithography with deformation-free pyrolysis and a GdCo coating to create a three-dimensional (3D) tripod structure that represents a building block of an 3D artificial spin ice, surrounded by a two-dimensional magnetic film. We map the three-dimensional magnetic configuration of the structure and its surroundings using soft x-ray magnetic laminography. In this way, we determine the magnetic configuration of the tripod nanostructure to be in the low-energy two-in-one-out spin ice state, observed at the 2D vertex of a kagome ice and predicted for three-dimensional vertices of magnetic buckyball structures. In contrast to isolated vertices, the degeneracy of this state can be lifted by the surrounding film, which also offers a route toward the controlled injection of emergent charges. This demonstration of the building block of a 3D spin system represents the first step toward the realization and understanding of more complex 3D artificial spin systems. - Ultra-high spin emission from antiferromagnetic FeRhItem type: Journal Article
Nature CommunicationsHamara, Dominik; Strungaru, Mara; Massey, Jamie; et al. (2024)An antiferromagnet emits spin currents when time-reversal symmetry is broken. This is typically achieved by applying an external magnetic field below and above the spin-flop transition or by optical pumping. In this work we apply optical pump-THz emission spectroscopy to study picosecond spin pumping from metallic FeRh as a function of temperature. Intriguingly we find that in the low-temperature antiferromagnetic phase the laser pulse induces a large and coherent spin pumping, while not crossing into the ferromagnetic phase. With temperature and magnetic field dependent measurements combined with atomistic spin dynamics simulations we show that the antiferromagnetic spin-lattice is destabilised by the combined action of optical pumping and picosecond spin-biasing by the conduction electron population, which results in spin accumulation. We propose that the amplitude of the effect is inherent to the nature of FeRh, particularly the Rh atoms and their high spin susceptibility. We believe that the principles shown here could be used to produce more effective spin current emitters. Our results also corroborate the work of others showing that the magnetic phase transition begins on a very fast picosecond timescale, but this timescale is often hidden by measurements which are confounded by the slower domain dynamics. - Stretched exponential magnetic relaxation dynamics in artificial square ice revealed through x-ray photon correlation spectroscopyItem type: Journal Article
Physical Review BScagnoli, Valerio; Skjærvø, Sandra H.; Massey, Jamie; et al. (2025)X-ray photon correlation scattering measurements are undertaken on a thermally active artificial spin ice based on the square lattice, referred to as artificial square ice, to probe the fluctuation timescales as a function of temperature as the system passes through the paramagnetic-antiferromagnetic phase transition, which belongs to the two-dimensional Ising universality class. In the paramagnetic regime, a single exponential timescale is seen, whereas at and below the critical temperature, a stretched exponential decorrelation is observed, with the stretching exponent decreasing from unity down to below one-half as the temperature reduces. This trend is confirmed by kinetic Monte Carlo simulations of a simplified point-dipolar square ice system, and is in agreement with past theoretical work on the kinetic Ising model where stretched exponential relaxation due to equilibrium domain wall dynamics below the critical temperature was found.
Publications 1 - 4 of 4