Perspective on design and technical challenges of Li-garnet solid-state batteries
OPEN ACCESS
Loading...
Author / Producer
Date
2022
Publication Type
Journal Article
ETH Bibliography
yes
Citations
Altmetric
OPEN ACCESS
Data
Rights / License
Abstract
Solid-state Li-ion batteries based on Li-garnet Li7La3Zr2O12 (LLZO) electrolyte have seen rapid advances in recent years. These solid-state systems are poised to address the urgent need for safe, non-flammable, and temperature-tolerant energy storage batteries that concomitantly possess improved energy densities and the cycle life as compared to conventional liquid-electrolyte-based counterparts. In this vision article, we review present research pursuits and discuss the limitations in the employment of LLZO solid-state electrolyte (SSE) for solid-state Li-ion batteries. Particular emphasis is given to the discussion of pros and cons of current methodologies in the fabrication of solid-state cathodes, LLZO SSE, and Li metal anode layers. Furthermore, we discuss the contributions of the LLZO thickness, cathode areal capacity, and LLZO content in the solid-state cathode on the energy density of Li-garnet solid-state batteries, summarizing their required values for matching the energy densities of conventional Li-ion systems. Finally, we highlight challenges that must be addressed in the move towards eventual commercialization of Li-garnet solid-state batteries.
Permanent link
Publication status
published
External links
Editor
Book title
Journal / series
Volume
23 (1)
Pages / Article No.
41 - 48
Publisher
Taylor & Francis
Event
Edition / version
Methods
Software
Geographic location
Date collected
Date created
Subject
Li-garnet solid-state batteries; LLZO solid-state electrolyte; Li metal anode; energy density; charge-storage capacity
Organisational unit
03934 - Kovalenko, Maksym / Kovalenko, Maksym